Nah that's not it. I guess it was on the TEG forums. Anyways, Desert Punk is a good one. Only 2 season though. Also Ninja Scroll is probably the best Anime movie ever next to Akira.
inb4 Light My Pyre, but: Neon Genesis Evangelion. Naruto if you want something light but serious at the same time. Other than that, my TODO list is huge, my TODO time, not so much...
Deadman Wonderland if you don't mind a little blood and gore. Eureka Seven is good. Code Geass is amazing. Katekyo Hitman Reborn is too. Hmmmm. Soul Eater if you can get past a little idiotic perversion. That about does it for my favorite anime list as far as I can remember. Stopped watching quite a while ago for whatever reason.
If you're looking for dubbed I would suggest Cowboy Bebop and Hetalia. Two of the only anime that even otakus will agree are better in English. (The Japanese Hetalia doesn't have the funny voices! That's the best part of the show!)
The Boondocks is much better than most anime because anime in general is repetitive, desudesu edgy garbage (PSG is an example, sorry.) The only one I'd recommend is dubbed Hetalia simply because it's funny.
As for anime movies, watch Ninja Scroll, Princess Mononoke, Paprika, Spirited Away and Perfect Blue. All awesome movies, I particularly enjoyed Perfect Blue (rumor has it Black Swan based his story on this anime).
Spirited away always scared me/made me sad back when it was showed on TV. God that was a good/creepy/sad movie.
I fail to see how Boondocks doesn't fall into repetitive edgy garbage. It's stupid stereotypical black people doing stupid stereotypical black things. EDIT: I can also vouch for the Studio Ghibli flicks.